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Humanity's uranium-238 inventory: A significant and enduring gamma-radiation liability Cover

Humanity's uranium-238 inventory: A significant and enduring gamma-radiation liability

Open Access
|May 2025

Figures & Tables

Fig. 1.

The U-238 decay-chain including gamma emissions. In parenthesis, the not-significant gamma from the decay of U-238 itself.
The U-238 decay-chain including gamma emissions. In parenthesis, the not-significant gamma from the decay of U-238 itself.

Fig. 2.

Secular equilibrium paths of the U-238 decay-chain.
Secular equilibrium paths of the U-238 decay-chain.

Fig. 3.

Evolution of the U-238 chain gamma dose-rate at the surface of an unshielded 238UO2-cylinder 40-cm-tall and 10-cm diameter. Pa-234m dominates at the start and for a few thousand years.
Evolution of the U-238 chain gamma dose-rate at the surface of an unshielded 238UO2-cylinder 40-cm-tall and 10-cm diameter. Pa-234m dominates at the start and for a few thousand years.

Fig. 4.

Gamma dose-rate from uncovered mill tailings as a function of time.
Gamma dose-rate from uncovered mill tailings as a function of time.

Estimated global-tailings U-238 and other relevant parameters

ParameterValue
Global tons of ore or tailings3 billion tons ore or tailings
Reference uranium content in ore0.15% (1.5 kg uranium/ton)
Fraction of U-238 in natural uranium99.3%
U-238 content per ton of ore1.4895 kg
Recovered U-238 per ton of ore1.2 kg
Unrecovered U-238 per ton of ore/tailing0.2895 kg
Conditioned U-2383.6 million tons
Tailings U-238868 500 tons
Recovery efficiency from ore80.6%

Humanity's U-238 inventory in metric tons and curies as of 2022

CategoryStock typeMetric tonsActivity (Curies)Percentage of total-mined (%)
Conditioned U-238 by stockLEU18 2526 1560.41
Reprocessed uranium127 00042 7992.84
Spent nuclear fuel363 000122 6318.4
DU3 100 0001 044 70069.24
Total conditioned U-238 3 608 2521 216 28680.6
Tailings U-238Mill-tailings868 500292 70019.4
Humanity's U-238Total-mined4 476 7521 507 984100

Global mill tailings estimates by source, date, and key concerns

ReferencesGlobal mill tailings estimateAnnual production estimateMajor regions affectedKey concerns
IAEA [17]Over 900 million cubic metersNot specifiedNorth America, Europe, AfricaRadon emissions, groundwater contamination, soil erosion
Sutherland [15]Over 1 billion metric tons in the year 2000 (sic)Over 200 million metric tons annuallyUnited States, Canada, former Soviet Union areasRadon release, groundwater contamination from in situ leaching
NEA [18]Over 1 billion metric tonsNot specifiedNorth America, Europe, Central AsiaLong-term containment, groundwater protection
NEA/IAEA Red Book [34]Over 1 billion metric tonsNot specifiedNorth America, Europe, Central AsiaRadon emissions, erosion, groundwater contamination

Observed gamma doses from uncovered mill-tailings

LocationGamma dose rate observedKey findings
Bellezane site, France [38]Above 10 μSv/h in certain areasGamma radiation levels vary by depth and exposure; higher values observed in specific areas emphasize the need for location-specific radiation mitigation strategies.
Tuyuk-Suu, Kyrgyzstan [39]10 μSv/h and higher in tailingsHighlights potential for elevated gamma exposure in legacy uranium processing regions, underscoring radiological risks in abandoned sites.
Former uranium mining sites, Portugal [40]Frequently exceeded 10 μSv/h, peaks at 20 μSv/hPersistent gamma dose rates on tailings surfaces present significant radiological hazards, necessitating ongoing monitoring and potential intervention.
Pridnieprovsky Chemical Plant, Ukraine [41]Up to 10 μSv/h in tailings and buildingsHigh gamma exposure levels detected in tailing areas and nearby structures suggest the need for targeted remediation in legacy milling sites.
Granitic uranium deposit, China [42]Average of 17.79 μSv/hTechnologically elevated gamma dose rates in a natural uranium-rich area high-light the potential for occupational and environmental exposure risks.
Uranium mining legacy sites, Portugal [43]7.5–9.5 μSv/h on tailings pilesGamma radiation from tailings poses long-term environmental and health risks, indicating the persistent impact of historical uranium mining.

Intensity-weighted gamma energy per decay and equilibrium contribution

IsotopeIntensity-weighted gamma energy per decay (keV)Contribution at equilibrium (%)
Pa-234m8.410.91
Ra-2266.100.66
Pb-214189.2920.49
Bi-2141076.4077.94
DOI: https://doi.org/10.2478/nuka-2025-0004 | Journal eISSN: 1508-5791 | Journal ISSN: 0029-5922
Language: English
Page range: 31 - 42
Submitted on: Dec 27, 2024
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Accepted on: Feb 10, 2025
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Published on: May 2, 2025
In partnership with: Paradigm Publishing Services
Publication frequency: 4 issues per year

© 2025 Claudio Pescatore, published by Institute of Nuclear Chemistry and Technology
This work is licensed under the Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 License.