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Meteoric CaO and carbon smoke particles collected in the upper stratosphere from an unanticipated source Cover

Meteoric CaO and carbon smoke particles collected in the upper stratosphere from an unanticipated source

Open Access
|Jan 2013

Figures & Tables

Fig. 1

Size distribution (microns) of the particles collected between 37 and 38.5 km during June 21–24, 2008 between ~72oN and ~78oN (modified after Della Corte et al., 2012).

Fig. 2

A FESEM image of pure carbon aggregate of numerous nanograins (D08_033) supported on the holey carbon film used for dust collection. The aggregate is about 300 nm in size. It is surrounded by a spray zone of smaller carbon nanograins.

Fig. 3

A FESEM image showing porous aggregate (D08_031) consisting of condensed Ca[O] nanograins that are accreted onto a larger melted aggregate of tiny carbonate grains. Small pores are visible in the largest sphere. The entire cluster is about 425 nm in size. The background is the holey carbon thin-film collection substrate.

Fig. 4

Lognormal size distributions for the condensed Ca[O] nanograins in aggregate particle D08_031 (Fig. 3) (solid squares) and the pure carbon nanograins in the aggregate smoke particle D08_033) (dots) and deposited on the support film (open circles) (Fig. 2) compared to the size distribution of Fe(Ni) nanometeorites collected in the lower stratosphere (diamonds) (Hemenway et al., 1961). All linear correlation coefficients (r 2) are ≥0.9.

Fig. 5

The Fe–C–O (at %) ternary diagram showing the composition of the porous smoke aggregate particle D08_031 (squares) and ‘in-hole’ analyses (circles) when the electron beam was placed across a hole in the holey carbon support film of the collector. These analyses represent a collector background composition. Iron in this diagram (diamond) results from a steel pin that is located directly below the actual collector (Ciucci, 2011; Ciucci et al., 2011). The open symbols are individual analyses; solid symbols are average compositions.

Fig. 6

A 610-nm nanosphere extracted from the dolomite decomposition experiment viewed in the FESEM used for this study to determine the collected grain compositions. The pores in this nanosphere are reminiscent of the outgassing pores in the largest sphere of porous aggregate particle (D08_031).

Table 1

Range of calcite grain sizes (microns) in selected CM meteorites

CM meteoriteSize range (µm)Y-79119820–80LAP 0479610–30Cold Bokkeveld20–90Nogoya20–70QUE 9300550–100QUE 8310020–80MET 0107010–60

[i] Sources: Benedix et al. (2003), De Leeuw et al. (2010) and Papike (1998).

Fig. 7

FESEM image of a composite pure carbon nanoparticle of a sphere resting on a platy substrate (D08-029) collected by DUSTER.

Language: English
Page range: 20174 - 20174
Submitted on: Nov 27, 2012
Published on: Jan 1, 2013
Published by: Stockholm University Press
In partnership with: Paradigm Publishing Services

© 2013 Vincenzo Della Corte, Franciscus J. M. Rietmeijer, Alessandra Rotundi, Marco Ferrari, Pasquale Palumbo, published by Stockholm University Press
This work is licensed under the Creative Commons Attribution 4.0 License.