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New particle formation in the presence of a strong biomass burning episode at a downwind rural site in PRD, China Cover

New particle formation in the presence of a strong biomass burning episode at a downwind rural site in PRD, China

Open Access
|Jan 2013

Figures & Tables

Fig. 1. 

Time series for (a) particle number size distributions and (b) sulphuric acid (H2SO4, blue empty dot), condensation sink (CS, green line with empty dot) and 15–25 nm particle number concentrations (N 15–25, red line) for the measurement period. The new particle formation event days are presented on a grey background. The x-axis is presented by DOY (day of year), 1 January is defined as day 1.

Table 1. Comparisons of various parameters between NPF event days and non-event days (during 9:00–12:00)

No. T (°C) RH (%) WS (m s−1) H2SO4 (107 cm−3) CS (10−2 s−1) H2SO4/CS (108 cm−3·s) NPF event 13 23±3.9 55±12 2.7±1.4 1.3±0.4 2.5±1.1 6.2±2.7 Non-event 17 27±3.0 67±8.3 1.9±1.4 0.9±0.5 3.0±1.2 3.7±2.4

Table 2. Comparisons of the condensation sink values with other studies at rural sites on NPF event days

Site Sampling period No. of events CS (×10−2 s−1) Ref. Kaiping Oct. 18–Nov. 16, 2008 12 0.3–8.6 This study Hyytiälä Winters 1997–2001 34 0.02–0.7 Kulmala et al. ( 2005) Po Valley 2002–2005 136 0.9–1.96 Hamed et al. ( 2007) K-puszta May 22–June 29, 2006 26 0.06–1.4 Yli-Juuti et al. ( 2009) Melpitz July, 2003–June, 2005 158 0.7 (mean) Jaatinen et al. ( 2009) Botsalano July 20, 2006–Feb. 5, 2008 988 0.4 (mean) Vakkari et al. (2011)
Fig. 2. 

The relationship between the number concentration of 15–25 nm particles and the ratio of sulphuric acid concentration to condensation sink. The data are from 09:00 to 12:00. NPF event days (red), Non-event days (blue).

Fig. 3. 

Time series of (a) particle number size distribution and the mean diameter of the dominating mode; (b) Temperature (T, red) and Relative Humidity (RH, blue); (c) Wind Speed (WS, orange) and Wind Direction (WD, green); (d) PM1 species concentrations; and (e) the ratio of primary emission to total mass concentration and fire count (pink) in PRD region during the episode.

Fig. 4. 

Time evolutions of (a) particle number size distributions and (b) particle volume size distributions during the episode. Different colour lines represent the mean distribution.

Fig. 5. 

The variations of (a) the relative contribution of different components, with PM1 mass concentration; (b) the relative contribution of particle number concentration in different modes, with primary species (BBOA and BC) mass concentration.

Fig. 6. 

Scatter plot of the total particle number concentration (N) versus the primary emissions (BBOA+BC). S 1 and S 2 indicate the lines of the minimum and maximum slopes which comprise the N-vs.-Pri. data, respectively.

Fig. 7. 

Time series of (a) N1 (black) and particle surface area concentration (blue); (b) N2 (red) and sulphuric acid concentration during the episode (green).

Language: English
Page range: 19965 - 19965
Submitted on: Oct 25, 2012
Accepted on: Jan 22, 2013
Published on: Jan 1, 2013
Published by: Stockholm University Press
In partnership with: Paradigm Publishing Services

© 2013 Z. B. Wang, M. Hu, D. L. Yue, L. Y. He, X. F. Huang, Q. Yang, J. Zheng, R. Y. Zhang, Y. H. Zhang, published by Stockholm University Press
This work is licensed under the Creative Commons Attribution 4.0 License.