A simple non-linear analytical relationship between aerosol accumulation number and sub-micron volume, explaining their observed ratio in the clean and polluted marine boundary layer
References
-
Ackerman
, A. S., Toon, 0. B. and Hobbs, P. 1994. Reas-sessing the dependence of cloud condensation nucleus concentration on formation rate., 445– 447. -
Bates
, T. S., Quinn, P. K., Covert, D. S., Coffman, D. J., Johnson, J. E.and Wiedensohler, A. 2000. Aerosol physical properties and controlling processes in the lower marine boundary layer: a comparison of sub-micron data from ACE1 and ACE2. Tellus, 258– 272. -
Bretherton
, C. S., Austin, P.and Siems, S. T. 1995. Cloudiness and marine boundary layer dynamics in the ASTEX Lagrangian experiments, II, cloudiness, drizzle, surface fluxes and etrainment.. 52, 5724– 2753. -
Fitzgerald
, J. W., Marti, J. J., Hoppel, W. A., Frick, G. M.and Gelbard, F. 1998. A one-dimensional sectional model to simulate multicomponent aerosol dynamics in the marine boundary layer (2). Model application. J. Geophys. Res. 103, 16103– 16117. -
Global Precipitation Climatology Project combined dataset
. 1999.http://www.dwd.de/research/gpcc. -
Hegg
, D. A.and Kaufman, Y. J. 1998. Measurements of the relationship between sub-micron aerosol number and volume concentration. J. Geophys. Res. 103, 5671– 5678. -
Hinds
, W. C. 1982. Aerosol technology, Wiley, New York. -
Hoell
, C., O'Dowd, C., Osborne, S.and Johnson, D. W. 2000. Timescale analysis of marine boundary layer aerosol evolution: Lagrangian case studies under clean and polluted cloudy conditions., 423- 438. -
Hoppel
, W. A., Fitzgerald, J. A.and Larson, R. E.. Aerosol size distributions in air masses advecting off the East Coast of the United States. J. Geophys. Res. 90, 2365– 2379. -
Hoppel
, W. A., Frick, G. M.and Larson, R. E. 1986. Effect of non-precipitating clouds on the aerosol size distribution in the marine boundary layer. Geophys. Res. Lett. 13, 125– 128. -
Hoppel
, W. A., Frick, G. M., Fitzgerald, J. W.and Larson, R. E. 1994. Marine boundary layer measure-ments of new particle formation and the effects nonpre-cipitating clouds have on the aerosol size distributions. J. Geophys. Res. 99, 14443– 14459. -
Hoppel
, W. A., Frick, G. M.and Fitzgerald, J. W. 1996. Deducing droplet concentration and supersaturation in marine boundary layer clouds from surface aerosol measurements. J. Geophys. Res. 101, 26553– 26565. -
Huffman
, G. J., Adler, R. F., Arkin, P. A., Chang, A., Ferraro, R., Gruber, A., Janowiak, J., McNab, A., Rudolf, B.and Schneider, U. 1997. The Global Precip-itation Climatology Project (GPCP) Combined Pre-cipitation Dataset. Bull. Americ. Meteor. Soc. 78, ( 1), 5– 20. -
Murphy
, D. M., Anderson, J. R., Quinn, P. K., McInnes, L. M., Brechtel, F. J., Kreidenweis, S. M., Middlebrook, A. M., Posfai, M., Thomson, D. S.and Buseck, P. R. 1998. Influence of sea-salt on aerosol radative properties in the Southern Ocean marine boundary layer. Nature, 62– 65. -
Neus.
, Weise,, Birmili,, Wex,, Wieden-sohler,and Covert,Size segregated chem-ical, gravimetric and number distribution derived mass closure of the aerosol in Sagres, Portugal during ACE-2. Tellus, 169– 184 -
O'Dowd
, C. D.and Smith, M. 1993. Physicochemical properties of aerosols over the Northeast Atlantic: evidence for wind-speed-related submicron sea-salt aerosol production. J. Geophys. Res. 98, 1137– 1149. -
Porter
, J. N.and Clarke, A. D. 1997. Aerosol size distri-bution models based on in situ measurements. J. Geo-phys. Res. 102, 6035– 6045. -
Pruppacher
, H. R.and Klett, J. D. 1978. Microphysics of clouds and precipitation . D. Reidel Publishing, Dordrecht. -
Putaud
, J.-P., Van Dingenen, R., Mangoni, M., Virkkula, A., Raes, F., Maring, H., Prospero, J. M., Swietlicki, E., Berg, O., Hillamo, R. and Makeld, T. 2000. Chem-ical mass closure and assessment of the origin of the submicron aerosol in the marine boundary layer and the free troposphere at Tenerife during ACE-2., 141– 168 -
Raes
, F. 1995. Entrainment of free tropospheric aerosols as a regulating mechanism for cloud condensation nuclei in the remote marine boundary layer. J. Geo-phys. Res. 100, 2893– 2903. -
Raes
, F., Van Dingenen, R., Cuevas, E., Van Velthoven, P. F. J.and Prospero, J. M. 1997. Observations of aerosols in the free troposphere and marine boundary layer of the subtropical north east Atlantic: discussion of processes determining their size distribution, J. Geo-phys. Res. 102, 21315– 21328. -
Raes
, F., Bates, T. S., McGovern, F. M., Van Liedekerke, M. 2000. The second Aerosol Characterisation Experi-ment: general overview and main results. Tellus, 111– 126. -
Seinfeld
, J. H.and Pandis, S. N. 1998. Atmospheric chem-istry and physics . Wiley, New York. -
Slinn
, W. G. N., Hasse, L., Hicks, B. B., Hogan, A. W., Lai, D., Liss, P. S., Munnich, K.O.., Sehmel, G. A. and Vittori, O. 1978. Some aspects of the transfer of atmo-spheric trace constituents past the air-sea interface.. 12, 2055– 2087 -
Van Dingenen
, R., Raes, F.and Jensen, N. 1995. Evidence for anthropogenic impact on number concentration and sulfate content of cloud-processed aerosol par-ticles over the North Atlantic. J. Geophys. Res. 100, 21057– 21067. -
Van Dingenen
, R., Raes, F., Putaud, J.-P., Virkkula, A.and Mangoni, M. 1999. Processes determining the relationship between aerosol number and non-sea-salt sulfate mass concentrations in the clean and perturbed marine boundary layer. J. Geophys. Res. 104, 8027– 8038. -
Verver
, G., Raes, F., Vogelezang, D.and Johnson, D. W. 2000. The second Aerosol Characterisation experi-ment: meteorological and chemical overview. Tellus, 126– 140.
DOI: https://doi.org/10.3402/tellusb.v52i2.16171 | Journal eISSN: 1600-0889
Language: English
Page range: 439 - 451
Submitted on: May 19, 1999
Accepted on: Sep 13, 1999
Published on: Jan 1, 2000
Published by: Stockholm University Press
In partnership with: Paradigm Publishing Services
© 2000 Rita Van Dingenen, Aki O. Virkkula, Frank Raes, Timothy S. Bates, Alfred Wiedensohler, published by Stockholm University Press
This work is licensed under the Creative Commons Attribution 4.0 License.