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Beyond a million years: Robust radiation shielding for high-level waste Cover

Beyond a million years: Robust radiation shielding for high-level waste

Open Access
|Aug 2025

Figures & Tables

Fig. 1.

Decay of VHLW from reprocessing 1 metric ton of SF (p. 17 in Ref. [1]).

Fig. 2.

Decay of activity content of 1 metric ton of Swedish SF (p. 16 in Ref. [3]).

Fig. 3.

External radiation 1 m away from 1 metric ton of Swedish SF (p. 23 in Ref. [3]).

Fig. 4.

Radiological dose rate, in Sv/h, 40 cm from two French HLW drill cores. The C2 drill core is VHLW; the CU1 drill core is SF (p. 533 in Ref. [5]).

Fig. 5.

The dose rate 2 cm away from a full-size, unshielded C2 cylinder as a function of time (Source, ANDRA).

Table 1.

Gamma dose rate (mSv/h) at three distances from a Pollux-8 cask loaded with eight PWR UO2 fuel assemblies, neglecting the shielding of the cask [2]

Decay time (million years)Surface (4 cm)Surface (2 cm extrapolated)
16.613.1
102.85.5
1002.75.4
10002.34.6
Table 2.

Dose rate (mSv/h) 2 cm from reference unshielded VHLW and SF at 1 million years [2]

Surface dose ratesC2 VHLW full-sizeC2 VHLW drill core8 PWR SF assembliesCU1 SF drill core
S2380.090.00325.40.82
S2340.180.00683.540.54
S23714.427.454.20.64
Total14.694.4613.142.00
Table 3.

Decay constants in per-million-year units

Chainλ
U-2381.55 × 10−5
Excess U-2342.82
Np-2370.324
Table 4.

Calculated shield thicknesses at 1 million years depending on each nuclear chain and using the proximity criterion. In bold are the required envelope thicknesses for each waste form. These values will decrease in time to reach the values for U-238, reported in italics

Surface dose ratesC2 VHLW full-sizeC2 VHLW drill core8 PWR SF assembliesCU1 SF drill core
S23816.661.941.1
S23424.357.336.5
S238 + S23428.867.546.7
S23753.548.143.528.2

[i] Dp = 0.02 mSv/h.

Table 5.

Calculated shield thicknesses at 1 million years depending on each nuclear chain and using the tolerability criterion. In bold are the required envelope thicknesses for each waste form. These values will decrease in time to reach the calculated for U-238, reported in italics

Surface dose ratesC2 VHLW full-sizeC2 VHLW drill core8 PWR SF assembliesCU1 SF drill core
S23842.15.287.466.6
S23449.813.582.761.9
S238 + S23454.317.893.072.2
S23772.266.962.246.9

[i] DT = 0.002 mSv/h.

Fig. 6.

Accrued, external dose from drill cores of several kinds of present and future French VHLW after a 10-min exposure, 40 cm from the drill core, and as a function of time (p. 352 in Ref. [9]).

DOI: https://doi.org/10.2478/nuka-2025-0009 | Journal eISSN: 1508-5791 (formerly 0029-5922) | Journal ISSN: 0029-5922
Language: English
Page range: 87 - 93
Submitted on: Oct 20, 2024
Accepted on: Feb 26, 2025
Published on: Aug 22, 2025
Published by: Institute of Nuclear Chemistry and Technology
In partnership with: Paradigm Publishing Services
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© 2025 Claudio Pescatore, published by Institute of Nuclear Chemistry and Technology
This work is licensed under the Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 License.